2,701 thoughts on “Silas Cook (Nov. 17)

  1. Carbon-carbon bond forming reactions being the basis of organic chemistry, this paper describes some very interesting reactions. You can get good yields, with incredibly less amount of time and very mild conditions. I would certainly love to hear the talk.

  2. I always have a soft spot in my heart when it comes to metal catalyzed reactions and research because working with the Rugen II catalyst (a Ruthenium based catalyst) was my area of research last year while I was an undergrad. This article focuses on the effectiveness of a an iron-catalyzed ortho-addition reaction, which I’m surprised even occurs due to the sterics of the overall reaction. One thing I was hoping to see, maybe because thats what I had previously worked on, was the kinetics of the reaction. I didn’t see much talk of experimental conditions or really any kinetic work. It always helps me to see how a reaction commences if there’s a FT-IR plot included in the article, just to show what order each reactant was, or if there was formation of any intermediates.

  3. I found this article pretty confusing, but I’m sure that’s because my knowledge of organic is quite limited. I can appreciate the benefit of a fast approach with good yields, since those two factors hinder a good number of experiments, especially seen in previous talks at colloquium. In the conclusion they have also given a small insight into what they will be working on next, understanding the mechanism better, which involves determining the turnover-limiting step.

  4. I’m not really a fan of Organic Chemistry nor do I really understand it, but the paper was sort of interesting. I can appreciate the need for finding an effective catalyst in these reactions, and how useful having fast, high-yield reactions are. A friend of mine doing organic research in the Ph.D. program at another university regularly runs reactions that take hours upon hours of time and he has frequent all-nighters to keep an eye on them, so I gather that speedy organic reactions that produce significant products are not usually standard. That’s pretty cool that this group has been able to develop those kinds of reactions, and I’m interested to hear what Dr. Cook has to say in his talk.

  5. This was a pretty advanced organic chemistry research article, and with the condensed “communication” format it wasn’t exactly easy to follow or understand every part. From what I can tell, the authors developed a new aromatic substitution reaction using an iron catalyst, and tested the effectiveness of their new method for a variety of electrophiles. Compared to previous methods, this new reaction is much faster and uses safe and inexpensive catalyst reagents.The content of this article was highly technical, but I thought still it was straight forward, even though I did not understand everything. One thing I thought would have improved the article was if there was some type of connection or brief discussion of applications this new methodology would be useful for. Meaning, what is the relevance of the electrophiles which were tested?

  6. I thought the article was pretty straightforward, but found myself very lost sometimes with the technicalities of the research. It is neat that they were able to a find new method for aromatic substitutions that are metal-catalyzed, faster, show great yields and are able to be tuned to accommodate a range of important electrophiles. But I agree with cody that they should’ve shown the relevance of these different electrophiles. Hopefully the talk will shed some light on that aspect.

  7. Though I am not really an organic enthusiast, the work in this article still seems pretty significant to me. They developed a highly selective, tunable pathway to alkylate a no so intuitive position. Great work, looking forward to the talk.

  8. It is important to be able to perform reactions with high selectivity in organic chemistry. This article discusses regioselective alkylation of a aminoquinoline at the ortho-position. Iron was used to catalyze the reaction.
    I was able to comprehend the study. The article discussed the work well. I think the talk today will be interesting. I’d like to see where the speaker will go with this topic.

  9. My feelings for organic chemistry are very similar to my feelings for biochemistry. I really have no interest for the subject at all. My biggest problem with this article was that the authors didn’t explain why the research was important or what it is used for. I like getting an understanding of the big picture since I am not as interested in the small details. I did find the quick reaction time and high yield pretty cool.

  10. Synthetic organic chemistry is definitely not my area, but still that didn’t make this article a tough read. It was easy to comprehend. Author talks about the development of a unified strategy of C-H alkylation reactions using iron as catalyst which helped them accommodate important electrophiles in the reaction, and they also managed to reduce reaction time and produce high yields. All in all a successful work, but I would certainly want the speaker to discuss more on the scope of this research.

  11. What a tiny paper! It was also very dense. I thought it was interesting that the ortho addition happened so fast and redaily despite the apparent steric hindrance in the molecule. I’m not a particular fan of metal catalyzed reactions but this one seems to go by without too much trouble at all. It was neat ending on a paper I could understand. Looking forward to the talk!

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